Plasmonic Nanostars as Efficient Broadband Scatterers for Random Lasing

نویسندگان

  • Johannes Ziegler
  • Christian Wörister
  • Cynthia Vidal
  • Calin Hrelescu
  • Thomas A. Klar
چکیده

Huge spectral coverage of random lasing throughout the visible up to the infrared range is achieved with star-shaped gold nanoparticles ("nanostars"). As intrinsically broadband scattering centers, the nanostars are suspended in solutions of various laser dyes, forming randomly arranged resonators which support coherent laser modes. The narrow emission line widths of 0.13 nm or below suggest that gold nanostars provide an efficient coherent feedback for random lasers over an extensive range of wavelengths, all together spanning almost a full optical octave from yellow to infrared.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Hybrid Multilayered Plasmonic Nanostars for Coherent Random Lasing

Here, we report that hybrid multilayered plasmonic nanostars can be universally used as feedback agents for coherent random lasing in polar or nonpolar solutions containing gain material. We show that silver-enhancement of gold nanostars reduces the pumping threshold for coherent random lasing substantially for both a typical dye (R6G) and a typical fluorescent polymer (MEH-PPV). Further, we re...

متن کامل

Plasmonic properties of single multispiked gold nanostars: correlating modeling with experiments.

Gold nanostars, possessing multiple sharp spikes, have emerged as promising plasmonic particles in the field of ultrasensitive sensing. We have developed a water-based method for high-yield synthesis of size-tunable anisotropic gold nanoparticles with a varying number of spiky surface protrusions, and performed systematic experimental and theoretical analyses of the optical properties of the si...

متن کامل

Size-Controlled Synthesis of Gold Nanostars and Their Characterizations and Plasmon Resonances

Gold nanostar particles were synthesized using seed-mediated method. Au-seed was synthesized with the diameter of approximately 3 nm and a considerably low STDEV of less than 1 nm. Then, different amount of Au seed was introduced into the growth solution of nanostars and the influence of the changes in concentration of Au seed on the growth process was investigated. The size of gold nanostars i...

متن کامل

Frequency behavior of coherent random lasing in diffusive resonant media

We investigate diffusive propagation of light and consequent random lasing in an amplifying medium comprising resonant spherical scatterers. A Monte-Carlo calculation based on photon propagation via three-dimensional random walks is employed to obtain the dwell-times of light in the system. We compare the inter-scatterer and intra-scatterer dwell-times for representative resonant and non-resona...

متن کامل

All-color plasmonic nanolasers with ultralow thresholds: autotuning mechanism for single-mode lasing.

We report on the first demonstration of broadband tunable, single-mode plasmonic nanolasers (spasers) emitting in the full visible spectrum. These nanolasers are based on a single metal-oxide-semiconductor nanostructure platform comprising of InGaN/GaN semiconductor nanorods supported on an Al2O3-capped epitaxial Ag film. In particular, all-color lasing in subdiffraction plasmonic resonators is...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:

دوره 3  شماره 

صفحات  -

تاریخ انتشار 2016